Ramón Cuadrado
Site-Resolved Contributions to the Magnetic-Anisotropy Energy and Complex Spin Structure of Fe/MgO Sandwiches
Cuadrado, Ramón; Oroszlány, László; Deák, András; Ostler, Thomas A.; Meo, Andrea; Chepulskii, Roman V.; Apalkov, Dmytro; Evans, Richard F.L.; Szunyogh, László; Chantrell, Roy W.
Authors
László Oroszlány
András Deák
Thomas A. Ostler
Andrea Meo
Roman V. Chepulskii
Dmytro Apalkov
Richard F.L. Evans
László Szunyogh
Roy W. Chantrell
Abstract
Fe/MgO-based magnetic tunnel junctions are among the most promising candidates for spintronic devices due to their high thermal stability and high tunneling magnetoresistance. Despite its apparent simplicity, the nature of the interactions between the Fe and MgO layers leads to complex finite-size effects and temperature-dependent magnetic properties which must be carefully controlled for practical applications. In this article, we investigate the electronic, structural, and magnetic properties of MgO/Fe/MgO sandwiches using first-principles calculations and atomistic spin modeling based on a fully parametrized spin Hamiltonian. We find a large contribution to the effective interfacial magnetic anisotropy from the two-ion exchange energy. Minimization of the total energy using atomistic simulations shows a surprising spin-spiral ground-state structure at the interface owing to frustrated ferromagnetic and antiferromagnetic interactions, leading to a reduced Curie temperature and strong layerwise temperature dependence of the magnetization. The different temperature dependences of the interface and bulklike layers results in an unexpected nonmonotonic temperature variation of the effective magnetic-anisotropy energy and temperature-induced spin-reorientation transition to an in-plane magnetization at low temperatures. Our results demonstrate the intrinsic physical complexity of the pure Fe/MgO interface and the role of elevated temperatures providing insight when interpreting experimental data of nanoscale magnetic tunnel junctions.
Citation
Cuadrado, R., Oroszlány, L., Deák, A., Ostler, T. A., Meo, A., Chepulskii, R. V., …Chantrell, R. W. (2018). Site-Resolved Contributions to the Magnetic-Anisotropy Energy and Complex Spin Structure of Fe/MgO Sandwiches. Physical Review Applied, 9(5), Article 054048. https://doi.org/10.1103/PhysRevApplied.9.054048
Journal Article Type | Article |
---|---|
Acceptance Date | Apr 25, 2018 |
Online Publication Date | May 30, 2018 |
Publication Date | 2018-05 |
Deposit Date | Jun 16, 2022 |
Journal | Physical Review Applied |
Print ISSN | 2331-7019 |
Electronic ISSN | 2331-7019 |
Publisher | American Physical Society |
Peer Reviewed | Peer Reviewed |
Volume | 9 |
Issue | 5 |
Article Number | 054048 |
DOI | https://doi.org/10.1103/PhysRevApplied.9.054048 |
Public URL | https://hull-repository.worktribe.com/output/4014991 |
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