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Two helices from one chiral centre - self organization of disc shaped chiral nanoparticles (2020)
Journal Article
Mehl, G. H., Yu, H., Qu, W., & Liu, F. (2021). Two helices from one chiral centre - self organization of disc shaped chiral nanoparticles. Chemical science, 12(5), 1778-1782. https://doi.org/10.1039/d0sc05100d

Gold nanoparticles (AuNPs) have been prepared and surface-functionalized with a mixture of 1-hexanethiol co-ligands and chiral discogen ligands separated from a disulfide functionviaa flexible spacer. Polarized optical microscopy together with differ... Read More about Two helices from one chiral centre - self organization of disc shaped chiral nanoparticles.

A Compact Full 2π Flexoelectro‐Optic Liquid Crystal Phase Modulator (2020)
Journal Article
Wang, X., Fells, J. A. J., Shi, Y., Ali, T., Welch, C., Mehl, G. H., Wilkinson, T. D., Booth, M. J., Morris, S. M., & Elston, S. J. (2020). A Compact Full 2π Flexoelectro‐Optic Liquid Crystal Phase Modulator. Advanced Materials Technologies, 5(12), Article 2000589. https://doi.org/10.1002/admt.202000589

Wavefront shaping, which is often achieved using liquid crystal (LC) spatial light modulators, is particularly important for a wide range of applications including laser microfabrication and micromanipulation, microscopy, and quantum optics. In this... Read More about A Compact Full 2π Flexoelectro‐Optic Liquid Crystal Phase Modulator.

Chirality enhancement in macro-chiral liquid crystal nanoparticles (2020)
Journal Article
Yu, H., Welch, C., Qu, W., Schubert, C. J., Liu, F., Siligardi, G., & Mehl, G. H. (2020). Chirality enhancement in macro-chiral liquid crystal nanoparticles. Materials Horizons, 7(11), 3021-3027. https://doi.org/10.1039/d0mh01274b

The amplification of molecular chirality by metal nanoparticles (NPs) is an important and rapidly evolving field in nanomaterial research with wide applications in smart materials, catalysis, and solvent-solute interactions. Here we present the resul... Read More about Chirality enhancement in macro-chiral liquid crystal nanoparticles.

Millisecond optical phase modulation using multipass configurations with liquid-crystal devices (2020)
Journal Article
Jin, Y., Elston, S. J., Fells, J. A., Booth, M. J., Welch, C., Mehl, G. H., & Morris, S. M. (2020). Millisecond optical phase modulation using multipass configurations with liquid-crystal devices. Physical Review Applied, 14(2), Article 024007. https://doi.org/10.1103/PhysRevApplied.14.024007

We present two configurations for analog 0 to 2π optical phase modulation using liquid crystals (LCs), each of which achieve switching times that are 1 ms or less. One configuration is based on the switching behavior of a so-called nematic pi cell, a... Read More about Millisecond optical phase modulation using multipass configurations with liquid-crystal devices.

Self-Assembly and Temperature-Driven Chirality Inversion of Cholesteryl-Based Block Copolymers (2020)
Journal Article
Krishnasamy, V., Qu, W., Chen, C., Huo, H., Ramanagul, K., Gothandapani, V., Mehl, G. H., Zhang, Q., & Liu, F. (2020). Self-Assembly and Temperature-Driven Chirality Inversion of Cholesteryl-Based Block Copolymers. Macromolecules, 53(11), 4193-4203. https://doi.org/10.1021/acs.macromol.9b02264

Block copolymers (BCPs), comprising a poly(methyl methacrylate) (PMMA) block and a poly(cholesteryloxyhexyl methacrylate) (PChMA) block, were synthesized via reversible addition–fragmentation chain transfer polymerization. The self-assembly of the li... Read More about Self-Assembly and Temperature-Driven Chirality Inversion of Cholesteryl-Based Block Copolymers.

Transmissive flexoelectro-optic liquid crystal optical phase modulator with 2 π modulation (2020)
Journal Article
Wang, X., Fells, J. A. J., Ali, T., Lin, J. D., Welch, C., Mehl, G. H., Wilkinson, T. D., Booth, M. J., Morris, S. M., & Elston, S. J. (2020). Transmissive flexoelectro-optic liquid crystal optical phase modulator with 2 π modulation. AIP Advances, 10(5), Article 055011. https://doi.org/10.1063/5.0009630

© 2020 Author(s). In this paper, we demonstrate analog phase modulation in a transmissive configuration using the flexoelectro-optic effect in short-pitch chiral nematic liquid crystal (LC) devices. Two different modes are considered, both of which a... Read More about Transmissive flexoelectro-optic liquid crystal optical phase modulator with 2 π modulation.

Temperature dependence of bend elastic constant in oblique helicoidal cholesterics (2020)
Journal Article
Iadlovska, O. S., Babakhanova, G., Mehl, G. H., Welch, C., Cruickshank, E., Strachan, G. J., Storey, J. M. D., Imrie, C. T., Shiyanovskii, S. V., & Lavrentovich, O. D. (2020). Temperature dependence of bend elastic constant in oblique helicoidal cholesterics. Physical Review Research, 2(1), Article 013238. https://doi.org/10.1103/PhysRevResearch.2.013248

Elastic moduli of liquid crystals, known as Frank constants, are of quintessential importance for understanding fundamental properties of these materials and for the design of their applications. Although there are many methods to measure the Frank c... Read More about Temperature dependence of bend elastic constant in oblique helicoidal cholesterics.

Analog modulation by the flexoelectric effect in liquid crystals (2020)
Journal Article
Yip, W. C., Welch, C., Mehl, G. H., & Wilkinson, T. D. (2020). Analog modulation by the flexoelectric effect in liquid crystals. Applied optics, 59(9), 2668-2673. https://doi.org/10.1364/AO.386096

We have solved the long-standing problems of stability and hysteresis, and we are able to obtain the homogeneous uniform lying helix structure in polymer-free cholesteric liquid crystals. This is instrumental for the present work to demonstrate the a... Read More about Analog modulation by the flexoelectric effect in liquid crystals.

Probing molecular ordering in the nematic phases of para-linked bimesogen dimers through NMR studies of flexible prochiral solutes (2020)
Journal Article
Heist, L. M., Samulski, E. T., Welch, C., Ahmed, Z., Mehl, G. H., Vanakaras, A. G., & Photinos, D. J. (2020). Probing molecular ordering in the nematic phases of para-linked bimesogen dimers through NMR studies of flexible prochiral solutes. Liquid crystals, 1-16. https://doi.org/10.1080/02678292.2019.1711214

The quadrupolar splittings of perdeuteriated n-decane dissolved in nematic phases formed by mesogenic dimers of the CBnCB series, for n = 7,9,10,11, are measured throughout the entire temperature range of these phases. These results are reported toge... Read More about Probing molecular ordering in the nematic phases of para-linked bimesogen dimers through NMR studies of flexible prochiral solutes.