Pickering emulsion-enhanced interfacial biocatalysis: tailored alginate microparticles act as particulate emulsifier and enzyme carrier

Yang, Xin; Wang, Yaolei; Bai, Ruixue; Ma, Hulin; Wang, Weihao; Sun, Hejia; Dong, Yuman; Qu, Fengmei; Tang, Qiming; Guo, Ting; Binks, Bernard P.; Meng, Tao

Abstract

A robust Pickering emulsion stabilized by lipase-immobilized alginate gel microparticles with a coating of silanized titania nanoparticles is developed for biphasic biocatalysis. The good recyclability and high stability of the proposed interfacial catalysis system have been verified, retaining about 90% of relative enzyme activity in 10 catalytic cycles with operation for 240 h. Meanwhile the Pickering emulsions remain stable during a storage time of one year. The green system can be widely applied to construct powerful platforms for enzyme or microorganism-driven interfacial catalysis.

Citation

Yang, X., Wang, Y., Bai, R., Ma, H., Wang, W., Sun, H., Dong, Y., Qu, F., Tang, Q., Guo, T., Binks, B. P., & Meng, T. (2019). Pickering emulsion-enhanced interfacial biocatalysis: tailored alginate microparticles act as particulate emulsifier and enzyme carrier. Green chemistry : an international journal and green chemistry resource : GC, 21(9), 2229-2233. https://doi.org/10.1039/c8gc03573c

• Journal Article Type: Article
• Acceptance Date: Jan 20, 2019
• Online Publication Date: Jan 23, 2019
• Publication Date: Jan 23, 2019
• Deposit Date: Feb 20, 2019
• Publicly Available Date: Jan 24, 2020
• Journal: Green Chemistry
• Print ISSN: 1463-9262
• Publisher: Royal Society of Chemistry
• Peer Reviewed: Peer Reviewed
• Volume: 21
• Issue: 9
• Pages: 2229-2233
• DOI: https://doi.org/10.1039/c8gc03573c
• Public URL: https://hull-repository.worktribe.com/output/1317590
• Publisher URL: https://pubs.rsc.org/en/content/articlelanding/2019/gc/c8gc03573c#!divAbstract
• Contract Date: Feb 20, 2019