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Simplification of detailed rate-based model of post-combustion CO₂ capture for full chain CCS integration studies

Oko, Eni; Wang, Meihong; Olaleye, Akeem K.

Authors

Eni Oko

Meihong Wang

Akeem K. Olaleye



Abstract

As post-combustion CO₂ capture (PCC) technology nears commercialisation, it has become necessary for the full carbon capture and storage (CCS) chain to be studied for better understanding of its dynamic characteristics. Model-based approach is one option for economically and safely reaching this objective. However, there is need to ensure that such models are reasonably simple to avoid the requirement for high computational time when carrying out such study. In this paper, a simplification approach for a detailed rate-based model of post-combustion CO₂ capture with solvents (rate-based mass transfer and reactions assumed to be at equilibrium) is presented. The simplified model can be used in model-based control and/or full chain CCS simulation studies. With this approach, we demonstrated significant reduction in CPU time (up to 60%) with reasonable model accuracy retained in comparison with the detailed model.

Citation

Oko, E., Wang, M., & Olaleye, A. K. (2015). Simplification of detailed rate-based model of post-combustion CO₂ capture for full chain CCS integration studies. Fuel, 142, 87-93. https://doi.org/10.1016/j.fuel.2014.10.083

Acceptance Date Oct 30, 2014
Online Publication Date Nov 11, 2014
Publication Date Feb 15, 2015
Deposit Date Mar 9, 2016
Publicly Available Date Mar 9, 2016
Journal Journal of further and higher education
Print ISSN 0016-2361
Publisher Elsevier
Peer Reviewed Peer Reviewed
Volume 142
Pages 87-93
DOI https://doi.org/10.1016/j.fuel.2014.10.083
Keywords Post-combustion carbon capture; Dynamic modelling; Model simplification; Steady state validation; Dynamic validation
Public URL https://hull-repository.worktribe.com/output/412573
Publisher URL http://www.sciencedirect.com/science/article/pii/S0016236114010849
Additional Information Author's accepted manuscript of article published in: Fuel, 2015, v.142
Contract Date Mar 9, 2016

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